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Second-order nonlinear optical properties of centrosymmetric nan...
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2021-02-10
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Hyper-Rayleigh scattering (HRS) technique has been used to study second-order nonlinear optical (NLO) properties of some centrosymmetric metal and semiconductor nanoparticles. All the samples display big "per particle" first hyperpolarizabilities 'beta'_(par). For centrosymmetric particles the contributions of multipolar radiations are very important to their second-order NLO responses. The metal nanoparticles show 'beta'_(par) two orders greater than that of the semiconductor ones, which can be
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